TY - JOUR
T1 - Antiferromagnetic real-space configuration probed by dichroism in scattered x-ray beams with orbital angular momentum
AU - McCarter, Margaret R.
AU - Saleheen, Ahmad I.U.
AU - Singh, Arnab
AU - Tumbleson, Ryan
AU - Woods, Justin S.
AU - Tremsin, Anton S.
AU - Scholl, Andreas
AU - De Long, Lance E.
AU - Hastings, J. Todd
AU - Morley, Sophie A.
AU - Roy, Sujoy
N1 - Publisher Copyright:
© 2023 American Physical Society.
PY - 2023/2/1
Y1 - 2023/2/1
N2 - X-ray beams with orbital angular momentum (OAM) are a promising tool for x-ray characterization techniques. Beams with OAM have a helicity - an azimuthally varying phase - which leads to a gradient of the light field. New material properties can be probed by utilizing the helicity of an OAM beam. Here, we demonstrate a dichroic effect in resonant diffraction from an artificial antiferromagnet with a topological defect. We found that the scattered OAM beam has circular dichroism at the antiferromagnetic Bragg peak whose sign is coupled to its helicity, which reveals the real-space configuration of the antiferromagnetic ground state. Thermal cycling of the artificial antiferromagnet can change the ground state, as indicated by reversal of the sign of circular dichroism. This result is one of the first demonstrations of a soft x-ray spectroscopy characterization technique utilizing the OAM of x rays. This helicity-dependent circular dichroism exemplifies the potential to utilize OAM beams to probe matter in a way that is inaccessible using currently available x-ray techniques.
AB - X-ray beams with orbital angular momentum (OAM) are a promising tool for x-ray characterization techniques. Beams with OAM have a helicity - an azimuthally varying phase - which leads to a gradient of the light field. New material properties can be probed by utilizing the helicity of an OAM beam. Here, we demonstrate a dichroic effect in resonant diffraction from an artificial antiferromagnet with a topological defect. We found that the scattered OAM beam has circular dichroism at the antiferromagnetic Bragg peak whose sign is coupled to its helicity, which reveals the real-space configuration of the antiferromagnetic ground state. Thermal cycling of the artificial antiferromagnet can change the ground state, as indicated by reversal of the sign of circular dichroism. This result is one of the first demonstrations of a soft x-ray spectroscopy characterization technique utilizing the OAM of x rays. This helicity-dependent circular dichroism exemplifies the potential to utilize OAM beams to probe matter in a way that is inaccessible using currently available x-ray techniques.
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U2 - 10.1103/PhysRevB.107.L060407
DO - 10.1103/PhysRevB.107.L060407
M3 - Article
AN - SCOPUS:85149679339
SN - 2469-9950
VL - 107
JO - Physical Review B
JF - Physical Review B
IS - 6
M1 - L060407
ER -