Abstract
The 4d-electron trimer lattice Ba₄Nb₁₋ₓRu₃₊ₓO₁₂ exhibits either a quantum spin liquid (QSL) or a heavy-fermion strange metal (HFSM) phase, depending on Nb content. In the QSL state, itinerant spinons act as effective heat carriers, enhancing thermal conductivity. Strikingly, applying a magnetic field up to 14 T causes an abrupt, up-to-5000% increase in heat capacity below 150 mK, disrupting the linear temperature dependence typical of both phases. Meanwhile, AC susceptibility and electrical resistivity remain nearly unchanged, while thermal conductivity drops by up to 40% below 4 K. These results suggest spinons, despite being charge-neutral, are highly sensitive to magnetic fields at low temperatures. We propose that the magnetic field could induce Anderson localization of spinons, creating emergent non-magnetic two-level systems responsible for the Schottky-like anomaly in heat capacity. These findings point to a previously unexplored regime of spinon dynamics, potentially governed by field-induced localization and distinct from conventional magnetic or transport signatures.
| Original language | English |
|---|---|
| Article number | 86 |
| Journal | npj Quantum Materials |
| Volume | 10 |
| Issue number | 1 |
| DOIs | |
| State | Published - Dec 2025 |
Bibliographical note
Publisher Copyright:© The Author(s) 2025.
Funding
G.C. thanks Xi Dai, Tai-Kai Ng, Feng Ye, Sandeep Sharma, Minhyea Lee and Longji Cui for useful discussions. Experimental work is supported by National Science Foundation via Grant No. DMR 2204811. Theoretical work by R.N. was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES) under Award # DE-SC0021346.
| Funders | Funder number |
|---|---|
| Office of Science Programs | |
| U.S. Department of Energy EPSCoR | |
| National Science Foundation Arctic Social Science Program | DMR 2204811 |
| DOE Basic Energy Sciences | DE-SC0021346 |
ASJC Scopus subject areas
- Electronic, Optical and Magnetic Materials
- Condensed Matter Physics