A spray-processable, low bandgap, and ambipolar donor - Acceptor conjugatedpolymer

Timothy T. Steckler; Xuan Zhang; Jungseek Hwang; Ryan Honeyager; Shino Ohira; Xiao Hong Zhang; Adrian Grant; Stefan Ellinger; Susan A. Odom; Daniel Sweat; David B. Tanner; Andrew G. Rinzler; Stephen Barlow; Jean Luc Brédas; Bernard Kippelen; Seth R. Marder; John R. Reynolds

doi:10.1021/ja809372u

A spray-processable, low bandgap, and ambipolar donor - Acceptor conjugatedpolymer

Timothy T. Steckler, Xuan Zhang, Jungseek Hwang, Ryan Honeyager, Shino Ohira, Xiao Hong Zhang, Adrian Grant, Stefan Ellinger, Susan A. Odom, Daniel Sweat, David B. Tanner, Andrew G. Rinzler, Stephen Barlow, Jean Luc Brédas, Bernard Kippelen, Seth R. Marder, John R. Reynolds

Chemistry

Producción científica: Article › revisión exhaustiva

218 Citas (Scopus)

Resumen

(Figure Presented) Combining a strong donor, tris(dodecyloxy)phenyl)- dithieno[3,2-b:2',3'-d]pyrrole, with a strong acceptor, 4,8-dithien-2-yl-2L4M2- benzo[1,2-c;4,5-c']bis[1,2,5]thiadiazole, has yielded the lowest bandgap, soluble, spray-processable polymer to date. The polymer has access to four different redox states and shows ambipolar behavior in OFETs. Multiple techniques, including transmission/absorption spectroscopy on SWCNTs and reflectance spectroscopy on gold were used to accurately estimate the optical bandgap at 0.5-0.6 eV, which correlates well to theoretical calculations.

Idioma original	English
Páginas (desde-hasta)	2824-2826
Número de páginas	3
Publicación	Journal of the American Chemical Society
Volumen	131
N.º	8
DOI	https://doi.org/10.1021/ja809372u
Estado	Published - mar 4 2009

ASJC Scopus subject areas

Catalysis
Biochemistry
General Chemistry
Colloid and Surface Chemistry

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10.1021/ja809372u

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Steckler, T. T., Zhang, X., Hwang, J., Honeyager, R., Ohira, S., Zhang, X. H., Grant, A., Ellinger, S., Odom, S. A., Sweat, D., Tanner, D. B., Rinzler, A. G., Barlow, S., Brédas, J. L., Kippelen, B., Marder, S. R., & Reynolds, J. R. (2009). A spray-processable, low bandgap, and ambipolar donor - Acceptor conjugatedpolymer. Journal of the American Chemical Society, 131(8), 2824-2826. https://doi.org/10.1021/ja809372u

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title = "A spray-processable, low bandgap, and ambipolar donor - Acceptor conjugatedpolymer",

abstract = "(Figure Presented) Combining a strong donor, tris(dodecyloxy)phenyl)- dithieno[3,2-b:2',3'-d]pyrrole, with a strong acceptor, 4,8-dithien-2-yl-2L4M2- benzo[1,2-c;4,5-c']bis[1,2,5]thiadiazole, has yielded the lowest bandgap, soluble, spray-processable polymer to date. The polymer has access to four different redox states and shows ambipolar behavior in OFETs. Multiple techniques, including transmission/absorption spectroscopy on SWCNTs and reflectance spectroscopy on gold were used to accurately estimate the optical bandgap at 0.5-0.6 eV, which correlates well to theoretical calculations.",

author = "Steckler, \{Timothy T.\} and Xuan Zhang and Jungseek Hwang and Ryan Honeyager and Shino Ohira and Zhang, \{Xiao Hong\} and Adrian Grant and Stefan Ellinger and Odom, \{Susan A.\} and Daniel Sweat and Tanner, \{David B.\} and Rinzler, \{Andrew G.\} and Stephen Barlow and Br{\'e}das, \{Jean Luc\} and Bernard Kippelen and Marder, \{Seth R.\} and Reynolds, \{John R.\}",

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doi = "10.1021/ja809372u",

language = "English",

volume = "131",

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Steckler, TT, Zhang, X, Hwang, J, Honeyager, R, Ohira, S, Zhang, XH, Grant, A, Ellinger, S, Odom, SA, Sweat, D, Tanner, DB, Rinzler, AG, Barlow, S, Brédas, JL, Kippelen, B, Marder, SR & Reynolds, JR 2009, 'A spray-processable, low bandgap, and ambipolar donor - Acceptor conjugatedpolymer', Journal of the American Chemical Society, vol. 131, n.º 8, pp. 2824-2826. https://doi.org/10.1021/ja809372u

TY - JOUR

T1 - A spray-processable, low bandgap, and ambipolar donor - Acceptor conjugatedpolymer

AU - Steckler, Timothy T.

AU - Zhang, Xuan

AU - Hwang, Jungseek

AU - Honeyager, Ryan

AU - Ohira, Shino

AU - Zhang, Xiao Hong

AU - Grant, Adrian

AU - Ellinger, Stefan

AU - Odom, Susan A.

AU - Sweat, Daniel

AU - Tanner, David B.

AU - Rinzler, Andrew G.

AU - Barlow, Stephen

AU - Brédas, Jean Luc

AU - Kippelen, Bernard

AU - Marder, Seth R.

AU - Reynolds, John R.

PY - 2009/3/4

Y1 - 2009/3/4

N2 - (Figure Presented) Combining a strong donor, tris(dodecyloxy)phenyl)- dithieno[3,2-b:2',3'-d]pyrrole, with a strong acceptor, 4,8-dithien-2-yl-2L4M2- benzo[1,2-c;4,5-c']bis[1,2,5]thiadiazole, has yielded the lowest bandgap, soluble, spray-processable polymer to date. The polymer has access to four different redox states and shows ambipolar behavior in OFETs. Multiple techniques, including transmission/absorption spectroscopy on SWCNTs and reflectance spectroscopy on gold were used to accurately estimate the optical bandgap at 0.5-0.6 eV, which correlates well to theoretical calculations.

AB - (Figure Presented) Combining a strong donor, tris(dodecyloxy)phenyl)- dithieno[3,2-b:2',3'-d]pyrrole, with a strong acceptor, 4,8-dithien-2-yl-2L4M2- benzo[1,2-c;4,5-c']bis[1,2,5]thiadiazole, has yielded the lowest bandgap, soluble, spray-processable polymer to date. The polymer has access to four different redox states and shows ambipolar behavior in OFETs. Multiple techniques, including transmission/absorption spectroscopy on SWCNTs and reflectance spectroscopy on gold were used to accurately estimate the optical bandgap at 0.5-0.6 eV, which correlates well to theoretical calculations.

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JF - Journal of the American Chemical Society

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A spray-processable, low bandgap, and ambipolar donor - Acceptor conjugatedpolymer

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